TY - JOUR
AU1 - Hertel, T.
AU2 - Fasel, R.
AU3 - Moos, G.
AB - We present a real-time investigation of ultra-fast carrier dynamics in single-wall carbon nanotube bundles using femtosecond time-resolved photoelectron spectroscopy. The experiments allow us to study the processes governing the sub-picosecond and the picosecond dynamics of non-equilibrium charge carriers. On the sub-picosecond time scale the dynamics are dominated by ultra-fast electron–electron scattering processes, which lead to internal thermalization of the laser-excited electron gas. We find that quasiparticle lifetimes decrease strongly as a function of their energy up to 2.38 eV above the Fermi level – the highest energy studied experimentally. The subsequent cooling of the laser-heated electron gas to the lattice temperature by electron–phonon interaction occurs on the picosecond time scale and allows us to determine the electron–phonon mass-enhancement parameter λ. The latter is found to be over an order of magnitude smaller if compared, for example, with that of a good conductor such as copper.
TI - Charge-carrier dynamics in single-wall carbon nanotube bundles: a time-domain study
JF - Applied Physics A: Materials Science Processing
DO - 10.1007/s003390201415
DA - 2002-10-01
UR - https://www.deepdyve.com/lp/springer-journals/charge-carrier-dynamics-in-single-wall-carbon-nanotube-bundles-a-time-Zuqt6EwcvR
SP - 449
EP - 465
VL - 75
IS - 4
DP - DeepDyve
ER -