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Planar visible–near infrared photodetectors based on organic–inorganic hybrid perovskite single crystal bulks

Planar visible–near infrared photodetectors based on organic–inorganic hybrid perovskite single... Single crystals of methylammonium lead trihalide perovskites have been widely applied in the research of next-generation photodetectors due to their remarkable light-harvesting properties, low trap density, and good carrier transport ability. Herein, the presented work demonstrates the high-quality and millimeter-scale single crystals CH3NH3PbBr3 and CH3NH3PbI3 perovskite-based planar photodetectors modified by the inverse temperature crystallization technique. The highest photoresponsivity of CH3NH3PbBr3 photodetector can reach ∼111 A W−1 under the visible illumination of 520 nm light and the highest photoresponsivity of CH3NH3PbI3 photodetector can reach ∼568 A W−1 under the infrared illumination of 895 nm light. The photodetectors also demonstrate high on/off ratio and fast response speed. It implies that CH3NH3PbBr3 and CH3NH3PbI3 single crystals based photodetectors reveal great attention for the applications of visible–infrared photodetection. http://www.deepdyve.com/assets/images/DeepDyve-Logo-lg.png Journal of Physics D: Applied Physics IOP Publishing

Planar visible–near infrared photodetectors based on organic–inorganic hybrid perovskite single crystal bulks

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Copyright
Copyright © 2020 IOP Publishing Ltd
ISSN
0022-3727
eISSN
1361-6463
DOI
10.1088/1361-6463/ab94e5
Publisher site
See Article on Publisher Site

Abstract

Single crystals of methylammonium lead trihalide perovskites have been widely applied in the research of next-generation photodetectors due to their remarkable light-harvesting properties, low trap density, and good carrier transport ability. Herein, the presented work demonstrates the high-quality and millimeter-scale single crystals CH3NH3PbBr3 and CH3NH3PbI3 perovskite-based planar photodetectors modified by the inverse temperature crystallization technique. The highest photoresponsivity of CH3NH3PbBr3 photodetector can reach ∼111 A W−1 under the visible illumination of 520 nm light and the highest photoresponsivity of CH3NH3PbI3 photodetector can reach ∼568 A W−1 under the infrared illumination of 895 nm light. The photodetectors also demonstrate high on/off ratio and fast response speed. It implies that CH3NH3PbBr3 and CH3NH3PbI3 single crystals based photodetectors reveal great attention for the applications of visible–infrared photodetection.

Journal

Journal of Physics D: Applied PhysicsIOP Publishing

Published: Jul 21, 2020

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