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- Publisher
- SPIE
- Copyright
- © 2013 Society of Photo-Optical Instrumentation Engineers (SPIE)
- Subject
- Research Papers
- ISSN
- 1934-2608
- eISSN
- 1934-2608
- DOI
- 10.1117/1.JNP.7.073090
- Publisher site
- See Article on Publisher Site
Abstract
Abstract. A monolithic quasi-solid-state dye-sensitized solar cell (DSSC) based on graphene-modified mesoscopic carbon-counter electrode is developed. A TiO 2 -working electrode layer, ZrO 2 spacer layer, and carbon counter electrode layer were constructed on a single conducting glass substrate by screen printing. The quasi-solid-state polymer gel electrolyte employed a polymer composite as the gelator, and effectively infiltrated the porous layers. Fabricated with normal carbon-counter electrode (NC-CE) containing graphite and carbon black, the DSSC had a power conversion efficiency (PCE) of 5.09% with the fill factor of 0.63 at 100 mW cm − 2 AM1.5 illumination. When the NC-CE was modified with graphene sheets, the PCE and fill factor were enhanced to 6.27% and 0.71, respectively. This improvement indicates excellent conductivity and high electrocatalytic activity of the graphene sheets, which have been considered as a promising platinum-free electrode material for DSSCs.
Journal
Journal of Nanophotonics – SPIE
Published: Jan 1, 2013