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References (35)
-
Lindner (2018)
Surface energy of corona treated PP, PE and PET films, its alteration as function of storage time and the effect of various corona dosages on their bond strength after laminationJ. Appl. Polym. Sci., 135
-
de Sousa (2021)
Management of plastic waste: A bibliometric mapping and analysisWaste Manage. Res., 39
-
Vanbergen (2020)
Recycling of Flexible Polyurethane Foam by Split‐Phase Alcoholysis: Identification of Additives and Alcoholyzing Agents to Reach Higher EfficienciesChemSusChem, 13
-
Ügdüler (2020)
Challenges and opportunities of solvent-based additive extraction methods for plastic recyclingWaste Manage., 104
-
G. Bolzon, G. Cornaggia, M. Shahmardani, A. Giampieri, A. Mameli (2015)
Beverages, 1
-
F. D. B. de Sousa (2021)
Waste Manage. Res., 39
-
Ügdüler (2021)
Towards a Better Understanding of Delamination of Multilayer Flexible Packaging Films by Carboxylic AcidsChemSusChem, 14
-
J. M. Garcia, M. L. Robertson (2017)
Science, 358
-
Žagar (2020)
Quantitative Determination of PA6 and/or PA66 Content in Polyamide-Containing WastesACS Sustainable Chem. Eng., 8
-
Walker (2020)
Recycling of multilayer plastic packaging materials by solvent-targeted recovery and precipitationSci. Adv., 6
-
Bolzon (2015)
Aluminum Laminates in Beverage Packaging: Models and ExperiencesBeverages, 1
-
E. Pauer, M. Tacker, V. Gabriel, V. Krauter (2020)
Clean. Environ. Syst., 1
-
Simón (2018)
Recycling of polyurethanes from laboratory to industry, a journey towards the sustainabilityWaste Manage., 76
-
S. Ügdüler, K. M. Van Geem, R. Denolf, M. Roosen, N. Mys, K. Ragaert, S. De Meester (2020)
Green Chem., 22
-
Sánchez-Rivera (2021)
Process intensification of solvent‐targeted recovery and precipitation (STRAP) of multilayer plastic packaging filmsChemSusChem, 14
-
Zahedifar (2021)
Multistage Chemical Recycling of Polyurethanes and Dicarbamates: A Glycolysis–Hydrolysis DemonstrationSustainability, 13
-
L. Ding, X. Zhang, Y. Wang (2020)
Coatings, 10
-
Tartakowski (2010)
Recycling of packaging multilayer films: New materials for technical productsResour., Conserv. Recycl., 55
-
E. Žagar, U. Češarek, A. Drinčić, S. Sitar, I. M. Shlyapnikov, D. Pahovnik (2020)
ACS Sustainable Chem. Eng., 8
-
Garcia (2017)
The future of plastics recyclingScience, 358
-
T. Vanbergen, I. Verlent, J. De Geeter, B. Haelterman, L. Claes, D. De Vos (2020)
ChemSusChem, 13
-
Moreno (2019)
Low-density polyethylene/polyamide 6 blends from multilayer films wasteJ. Appl. Polym. Sci., 136
-
P. Zahedifar, L. Pazdur, C. M. L. Vande Veld, P. Billen (2021)
Sustainability, 13
-
T. W. Walker, N. Frelka, Z. Shen, A. K. Chew, J. Banick, S. Grey, M. S. Kim, J. A. Dumesic, R. C. Van Lehn, G. W. Huber (2020)
Sci. Adv., 6
-
Pauer (2020)
Sustainability of flexible multilayer packaging: Environmental impacts and recyclability of packaging for bacon in blockClean. Environ. Syst., 1
-
M. R. Robertson, C. Klimas (2019)
DePaul Discoveries, 8
-
D. Simón, A. M. Borreguero, A. de Lucas, J. F. Rodríguez (2018)
Waste Manage., 76
-
C. Morales-Caselles, J. Viejo, E. Martí, D. González-Fernández, H. Pragnell-Raasch, J. I. González-Gordillo, E. Montero, G. M. Arroyo, G. Hanke, V. S. Salvo, O. C. Basurko, N. Mallos, L. Lebreton, F. Echevarría, T. van Emmerik, C. M. Duarte, J. A. Gálvez, E. van Sebille, F. Galgani, C. M. García, P. S. Ross, A. Bartual, C. Ioakeimidis, G. Markalain, A. Isobe, A. Cózar (2021)
Nat. Sustain., 4
-
Ügdüler (2020)
Towards closed-loop recycling of multilayer and coloured PET plastic waste by alkaline hydrolysisGreen Chem., 22
-
Civancik-Uslu (2021)
Moving from linear to circular household plastic packaging in Belgium: Prospective life cycle assessment of mechanical and thermochemical recyclingResour., Conserv. Recycl., 171
-
Morales-Caselles (2021)
An inshore–offshore sorting system revealed from global classification of ocean litterNat. Sustain., 4
-
M. Lindner, N. Rodler, M. Jesdinszki, M. Schmid, S. Sängerlaub (2018)
J. Appl. Polym. Sci., 135
-
V. Engineering, M. Technology, C. Goods (2020)
Kunstoffe International
-
D. Civancik-Uslu, T. T. Nhu, B. Van Gorp, U. Kresovic, M. Larrain, P. Billen, K. Ragaert, S. De Meester, J. Dewulf, S. Huysveld (2021)
Resour., Conserv. Recycl., 171
-
Ügdüler (2022)
Analysis of the kinetics, energy balance and carbon footprint of the delamination of multilayer flexible packaging films via carboxylic acidsResour., Conserv. Recycl., 181
- Publisher
- Royal Society of Chemistry
- Copyright
- © Royal Society of Chemistry 2024 Registered charity number: 207890
- eISSN
- 1463-9270
- DOI
- 10.1039/d2gc01531e
- Publisher site
- See Article on Publisher Site
Abstract
Recycling of multilayer packaging is challenging due to the heterogeneity of plastic types that can be comingled by chemical bonding with adhesives. For this purpose, delamination of polyamide(PA)/polyolefin (PO) multilayers, glued together by polyurethane (PUR), was investigated. A previous method, using solvent targeted dissolution-precipitation (STRAP) for fractionation of the outer plastic layers (PO or PA) gave mixed fractions. In contrast, specifically targeting the PUR adhesive by glycolysis-depolymerization accomplished highly selective separation. A single processing step at mild temperatures in sustainable solvents based on ethylene glycol oligomers, detached the PA from the PO fraction, leading to split films without impurities. This study is the first of its kind to analyze the chemistry of delamination in depth and introduces a process that could be generally applicable for a multitude of other multilayers that are bonded by PUR adhesives.
Journal
Green Chemistry – Royal Society of Chemistry
Published: Sep 20, 2022