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- Publisher
- Wiley
- Copyright
- © 2022 Wiley‐VCH GmbH
- ISSN
- 1616-301X
- eISSN
- 1616-3028
- DOI
- 10.1002/adfm.202209743
- Publisher site
- See Article on Publisher Site
Abstract
High electrocatalytic activity with tunable luminescence is crucial for the development of electrochemiluminescence (ECL) luminophores. In this study, a porphyrin‐based heterobimetallic 2D metal organic framework (MOF), [(ZnTCPP)Co2(MeIm)] (1), is successfully self‐assembled from the zinc(II) tetrakis(4‐carboxyphenyl)porphine (ZnTCPP) linker and cobalt(II) ions in the presence of 2‐methylimidazole (MeIm) by a facile one‐pot reaction in methanol at room temperature. On the basis of the experimental results and the theoretical calculations, the MOF 1 contains paddle–wheel [Co2(‐CO2)4] secondary building units (SBUs) axially coordinated by a MeIm ligand, which is very beneficial to the electron transfer between the Co(II) ions and oxygen. Combining the photosensitizers ZnTCPP and the electroactive [Co2(‐CO2)4] SBUs, the 2D MOF 1 possesses an excellent ECL performance, and can be used as a novel ECL probe for rapid nonamplified detection of the RdRp gene of SARS‐CoV‐2 with an extremely low limit of detection (≈30 aM).
Journal
Advanced Functional Materials – Wiley
Published: Nov 1, 2022
Keywords: axial coordinations; ECL probes; heterobimetallic 2D MOFs; porphyrin; SARS‐CoV‐2