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Abstract
A novel Layered@Spinel@Carbon heterostructure is successfully fabricated via an in situ synchronous carbonization-reduction process based on a bio-inspired coating method, which comprises a core of Li-rich layered (R3̄m) oxide, a spinel phase (Fd3̄m) interlayer and a carbon nano-coating. This unique structure, which combines the advantages of the high capacity Li-rich layered structure, 3D fast Li+ diffusion channels of the spinel structure and the high conductivity of the carbon coating, shows extremely high discharge capacity (as high as 334.5 mA h g−1) and superior rate capability. This strategy may provide some new insights into the design and synthesis of various electrode materials for high performance energy storage devices.
Journal
Journal of Materials Chemistry A – Royal Society of Chemistry
Published: Feb 3, 2015